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New quinazolinone-thiazolidinedione hybrids as selective anti-lung cancer agents and promising EGFR inhibitors.

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Future medicinal chemistry 📖 저널 OA 75% 2025: 6/6 OA 2026: 24/34 OA 2025~2026 2026 Vol.18(4) p. 415-428
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Tokalı P, Şenol AM, Ateşoğlu Ş, Çakır F, Şenol H, Tokali FS

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[AIM] Lung cancer remains a leading cause of cancer-related deaths, largely due to therapy resistance and toxicity.

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APA Tokalı P, Şenol AM, et al. (2026). New quinazolinone-thiazolidinedione hybrids as selective anti-lung cancer agents and promising EGFR inhibitors.. Future medicinal chemistry, 18(4), 415-428. https://doi.org/10.1080/17568919.2026.2620368
MLA Tokalı P, et al.. "New quinazolinone-thiazolidinedione hybrids as selective anti-lung cancer agents and promising EGFR inhibitors.." Future medicinal chemistry, vol. 18, no. 4, 2026, pp. 415-428.
PMID 41636324 ↗

Abstract

[AIM] Lung cancer remains a leading cause of cancer-related deaths, largely due to therapy resistance and toxicity. This study develops novel quinazolinone-thiazolidinedione (TZD) hybrids by combining two anticancer pharmacophores to achieve more selective and potent EGFR inhibitors.

[MATERIALS AND METHODS] A total of 14 quinazolinone-TZD hybrids were synthesized and characterized. Their cytotoxicity was evaluated in A549 lung adenocarcinoma and BEAS-2B normal bronchial cells. EGFR binding was analyzed via molecular docking and MM-GBSA, with 500 ns molecular dynamics simulations supporting the stability of selected complexes. ADME predictions assessed drug-likeness and oral bioavailability.

[RESULTS] Several compounds showed selective cytotoxicity against A549 cells, with compound 9 (thiophen-2-ylmethyl substituent) emerging as the most active (IC = 3.85 μM, SI = 36.0), outperforming gefitinib (IC = 9.59 μM, SI = 1.9) and exhibiting higher selectivity than sorafenib (IC = 3.24 μM, SI = 5.4). Computational analyses revealed key interactions with EGFR residues (Cys-797, Arg-841, Asn-842, and Phe-997), supported by stable molecular dynamics behavior and favorable ADME predictions.

[CONCLUSION] These findings indicate that the synthesized hybrids, particularly compound , represent promising leads for selective EGFR-targeted lung cancer therapy and support further optimization.

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